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Palladium-catalyzed asymmetric allylic substitutions by axially chiral P,S-, S,S-, and S,O-heterodonor ligands with a binaphthalene framework
其他题名Palladium-Catalyzed Asymmetric Allylic Substitutions by Axially Chiral P,S-; S,S-; and S,O-Heterodonor Ligands with Binaphthalene Framework.
Shi M(施敏); Zhang W(张雯); Shi M(施敏)
2004
发表期刊Tetrahedron-Asymmetry
卷号15期号:19页码:3161-3169
摘要Axially chiral P,S-heterodonor ligand L1 is effective in the asymmetric allylic substitution of 1,3-diphenylpropenyl acetate with dimethyl malonate. its bidentate coordination pattern to a I'd metal center with both P and S atoms has been unambiguously established by X-ray diffraction and NMR spectroscopic analyses. Herein, we further disclose that axially chiral S,S-heterodonor ligands L2-L4 are also effective in the same reaction to give the allylic alkylation product in moderate to good ee. However, the corresponding S,O-heterodonor ligands are not as effective as the corresponding P,S- or S,S-heterodonor ligands in the same asymmetric reaction. (C) 2004 Elsevier Ltd. All rights reserved.
学科领域金属有机化学
部门归属中国科学院上海有机化学研究所金属有机化学国家重点实验室
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收录类别SCI
语种英语
WOS记录号WOS:000224447500020
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被引频次:19[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.sioc.ac.cn/handle/331003/9940
专题金属有机化学国家重点实验室
通讯作者Shi M(施敏)
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GB/T 7714
Shi M,Zhang W,Shi M. Palladium-catalyzed asymmetric allylic substitutions by axially chiral P,S-, S,S-, and S,O-heterodonor ligands with a binaphthalene framework[J]. Tetrahedron-Asymmetry,2004,15(19):3161-3169.
APA Shi M,Zhang W,&施敏.(2004).Palladium-catalyzed asymmetric allylic substitutions by axially chiral P,S-, S,S-, and S,O-heterodonor ligands with a binaphthalene framework.Tetrahedron-Asymmetry,15(19),3161-3169.
MLA Shi M,et al."Palladium-catalyzed asymmetric allylic substitutions by axially chiral P,S-, S,S-, and S,O-heterodonor ligands with a binaphthalene framework".Tetrahedron-Asymmetry 15.19(2004):3161-3169.
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