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学科主题: 高分子化学
题名: Carbazolo[2,1-a]carbazole Diimide: A Building Block for Organic Electronic Materials
其他题名: 咔唑并咔唑二酰亚胺: 有机电子材料的一类新的构筑单元
作者: Zhao Z(赵征)1; Wang ZL(王中丽)1; Zhang X(张旭)1; Gao SM(高思敏)1; Yang XD(杨笑迪)1; Duan ZM(段智明)1; Gao XK(高希珂)1
通讯作者: 杨笑迪 ; 高希珂
刊名: ChemPlusChem
发表日期: 2015
DOI: 10.1002/cplu.201402360
卷: 80, 期:1, 页:57-61
收录类别: SCI
文章类型: 论文
英文摘要: A new class of carbazolo[2,1-a]carbazole diimide compounds (CBZCBZ-DI, 3) are designed and synthesized. The synthesis, X-ray crystal structure, absorption spectra, and electrochemical properties of 3 as well as the charge transport properties are investigated. Theoretical calculation is also carried out based on the X-ray crystal structure of 3a to understand the relationship between the structure and the charge transport properties. Single-crystal X-ray analysis revealed that the molecules of 3a adopt a slipped face-to-face pi-stacking mode with a large intermolecular pi-overlap and an interplanar distance of 3.4 angstrom. Crystalline transistors of 3a display high hole mobility of 0.5 cm(2)V(-1) s(-1), which is among the highest reported mobility values for carbazole-based N-heteroacenes. Two useful brominated derivatives (4, 5) are also prepared for synthesizing more new pi-functional materials.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000348721900008
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39836
Appears in Collections:高分子材料研究室_期刊论文

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作者单位: 1.中科院上海有机化学研究所, 有机功能分子合成与组装化学重点实验室
2.复旦大学
3.上海大学

Recommended Citation:
Zhao Z,Wang ZL,Zhang X,et al. Carbazolo[2,1-a]carbazole Diimide: A Building Block for Organic Electronic Materials[J]. ChemPlusChem,2015,80(1):57-61.
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