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学科主题: 金属有机化学
题名: Chiral phosphine-catalyzed tunable cycloaddition reactions of allenoates with benzofuranone-derived olefins for a highly regio-, diastereo- and enantioselective synthesis of spiro-benzofuranones
其他题名: 手性膦催化的高区域和高对映选择性环化反应研究-构建螺环骨架的苯并呋喃类化合物
作者: Wang D(王德)1; Wang GP(王国鹏)1; Sun YL(孙姚良)1; Zhu SF(朱守非)1; Wei Y(魏音)1; Zhou QL(周其林)1; Shi M(施敏)1
通讯作者: 魏音 ; 周其林 ; 施敏
刊名: Chem. Sci.
发表日期: 2015
DOI: 10.1039/c5sc03135d
卷: 6, 期:12, 页:7319-7325
收录类别: SCI
文章类型: 论文
英文摘要: The first regioselective catalytic asymmetric [3 + 2] cycloaddition of benzofuranone-derived olefins with allenoates and substituted allenoates has been developed in the presence of (R)-SITCP, affording different functionalized 3-spirocyclopentene benzofuran-2-ones in good yields with high enantioselectivities under mild conditions. The substrate scope has also been examined. The regioselective outcomes for this phosphine-catalyzed [3 + 2] cycloaddition reaction can be rationalized using DFT calculations.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000365225300076
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39672
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 1.中科院上海有机化学研究所, 金属有机化学国家重点实验室
2.南开大学

Recommended Citation:
Wang D,Wang GP,Sun YL,et al. Chiral phosphine-catalyzed tunable cycloaddition reactions of allenoates with benzofuranone-derived olefins for a highly regio-, diastereo- and enantioselective synthesis of spiro-benzofuranones[J]. Chem. Sci.,2015,6(12):7319-7325.
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