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Gold(I)-catalyzed cycloisomerization of vinylidenecyclopropane-enes via carbene or non-carbene processes
Alternative Title金催化的亚乙烯基环丙烷的环异构化反应
Li DY(李德尧)1; Wei Y(魏音)1; MAREK ILAN1; Tang XY(唐翔鹰)1; Shi M(施敏)1
2015
Source PublicationChem. Sci.
Volume6Issue:10Pages:5519-5525
AbstractGold catalyzed cycloisomerization of aromatic ring tethered vinylidenecyclopropane-enes provides a divergent synthetic protocol for the construction of O-containing fused heterocycles through controllable carbene or non-carbene related processes. The carbene induced process features a new amphiphilic strategy to generate a gold carbene via a rearrangement of vinylidenecyclopropane. Whereas, the electronic effect of the ortho-substituents switches the reaction mode onto the non-carbene related process, from which five-or six-membered rings are selectively produced through allyl-migration.
Subtype论文
Subject Area金属有机化学
DOI10.1039/c5sc01806d
URL查看原文
Indexed BySCI
Language英语
WOS IDWOS:000361212000020
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Document Type期刊论文
Identifierhttp://ir.sioc.ac.cn/handle/331003/39639
Collection金属有机化学国家重点实验室
Corresponding AuthorTang XY(唐翔鹰); Shi M(施敏)
Affiliation1.中科院上海有机化学研究所, 金属有机化学国家重点实验室
2.以色列理工学院
Recommended Citation
GB/T 7714
Li DY,Wei Y,MAREK ILAN,et al. Gold(I)-catalyzed cycloisomerization of vinylidenecyclopropane-enes via carbene or non-carbene processes[J]. Chem. Sci.,2015,6(10):5519-5525.
APA 李德尧,魏音,MAREK ILAN,唐翔鹰,&施敏.(2015).Gold(I)-catalyzed cycloisomerization of vinylidenecyclopropane-enes via carbene or non-carbene processes.Chem. Sci.,6(10),5519-5525.
MLA 李德尧,et al."Gold(I)-catalyzed cycloisomerization of vinylidenecyclopropane-enes via carbene or non-carbene processes".Chem. Sci. 6.10(2015):5519-5525.
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