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学科主题: 金属有机化学
题名: Palladium-Catalyzed Intramolecular Aminoacetoxylation of Unactivated Alkenes with Hydrogen Peroxide as Oxidant
其他题名: 钯催化非活性烯烃的分子内胺乙酰基化反应
作者: Zhu HT(朱海涛); Chen PH(陈品红); Liu GS(刘国生)
通讯作者: 刘国生
刊名: Org. Lett.
发表日期: 2015
DOI: 10.1021/acs.orglett.5b00373
卷: 17, 期:6, 页:1485-1488
收录类别: SCI
文章类型: 论文
英文摘要: A palladium-catalyzed intramolecular aminoacetoxylation of unactivated alkenes was developed in which H2O2 was used as the sole oxidant. A variety of 3-acetoxylated piperidines were obtained in good yields with good to excellent regio- and diastereoselectivities. Mechanistic study revealed that the addition of di(2-pyridyl) ketone (dpk) ligand was crucial to promote the oxidative cleavage of the C-Pd(II) bond by H2O2 to give the C-OAc bond.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000351558100035
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39585
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所, 金属有机化学国家重点实验室

Recommended Citation:
Zhu HT,Chen PH,Liu GS. Palladium-Catalyzed Intramolecular Aminoacetoxylation of Unactivated Alkenes with Hydrogen Peroxide as Oxidant[J]. Org. Lett.,2015,17(6):1485-1488.
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