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学科主题: 金属有机化学
题名: Rhodium-catalyzed C-H functionalization-based approach to eight-membered lactams
其他题名: 铑催化的通过C-H键活化合成八元内酰胺的方法
作者: Wu SZ(吴尚泽)1; Ceng R(曾荣)1; Fu CL(傅春玲)1; Yu YH(余亦华)1; Zhang X(张雪)1; Ma SM(麻生明)1
通讯作者: 张雪 ; 麻生明
刊名: Chem. Sci.
发表日期: 2015
DOI: 10.1039/c5sc00092k
卷: 6, 期:4, 页:2275-2285
收录类别: SCI
文章类型: 论文
英文摘要: A Rh(III) catalyzed formal [4 + 2 + 2] cyclization of N-pivaloyloxybenzamides 1 with 1,6-allene-enes 2 by C-H functionalization is reported. The reactions occur at room temperature and are compatible with air and moisture with a tolerance of many synthetically useful functional groups. The follow-up modifications of the products have been demonstrated. After careful mechanistic studies and DFT calculation, a reaction mechanism was proposed.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000351412800016
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39584
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 1.浙江大学
2.中科院上海有机化学研究所, 金属有机化学国家重点实验室

Recommended Citation:
Wu SZ,Ceng R,Fu CL,et al. Rhodium-catalyzed C-H functionalization-based approach to eight-membered lactams[J]. Chem. Sci.,2015,6(4):2275-2285.
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