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学科主题: 金属有机化学
题名: Rh-II-Catalyzed [3+2] Cycloaddition of 2H-Azirines with N-Sulfonyl-1,2,3-Triazoles
其他题名: 铑(II)催化的氮杂三元环和三氮唑的[3+2]环加成反应
作者: Zhao YZ(赵允州); Yang HB(杨海斌); Tang XY(唐翔鹰); Shi M(施敏)
通讯作者: 唐翔鹰 ; 施敏
刊名: Chem.-Eur. J.
发表日期: 2015
DOI: 10.1002/chem.201406460
卷: 21, 期:9, 页:3562-3566
收录类别: SCI
文章类型: 论文
英文摘要: Rh-II-catalyzed intermolecular [3+2] cycloaddition of 2H-azirines with N-sulfonyl-1,2,3-triazoles is disclosed, in which a series of fully functionalized pyrroles is produced via rhodium azavinyl carbene intermediates. A distinct feature of this reaction is that the azavinyl carbene serves as a [2C] equivalent, instead of as [1C] or aza-[3C] synthons, which have been reported previously in cyclopropanations and [3+n] cycloadditions. Moreover, this methodology has also been successfully applied in the total synthesis of URB447 as well as the formal synthesis of Atorvastatin (Lipitor).
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000350116200010
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39580
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所, 金属有机化学国家重点实验室

Recommended Citation:
Zhao YZ,Yang HB,Tang XY,et al. Rh-II-Catalyzed [3+2] Cycloaddition of 2H-Azirines with N-Sulfonyl-1,2,3-Triazoles[J]. Chem.-Eur. J.,2015,21(9):3562-3566.
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