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学科主题: 金属有机化学
题名: Highly Enantioselective Nickel-Catalyzed Intramolecular Reductive Cyclization of Alkynones
其他题名: 高立体选择性的分子内炔酮的还原环化
作者: Fu WZ(付文振); Nie M(聂明); Wang AZ(王爱珍); Cao ZP(曹子平); Tang WJ(汤文军)
通讯作者: 汤文军
刊名: Angew. Chem.-Int. Edit.
发表日期: 2015
DOI: 10.1002/anie.201410700
卷: 54, 期:8, 页:2520-2524
收录类别: SCI
文章类型: 论文
英文摘要: The first asymmetric nickel-catalyzed intramolecular reductive cyclization of alkynones is reported. A P-chiral monophosphine and triethylsilane were used as the ligand and the reducing reagent, respectively, to form a series of tertiary allylic alcohols bearing furan/pyran rings in excellent yields and enantioselectivities. This reaction has a broad substrate scope and enabled the efficient synthesis of dehydroxycubebin and chiral dibenzocyclooctadiene skeletons.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000350100000040
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39569
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所, 生命有机化学国家重点实验室

Recommended Citation:
Fu WZ,Nie M,Wang AZ,et al. Highly Enantioselective Nickel-Catalyzed Intramolecular Reductive Cyclization of Alkynones[J]. Angew. Chem.-Int. Edit.,2015,54(8):2520-2524.
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