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学科主题: 金属有机化学
题名: Highly Regio- and Enantioselective Synthesis of N-Substituted 2-Pyridones: Iridium-Catalyzed Intermolecular Asymmetric Allylic Amination
其他题名: 金属铱催化的不对称烯丙基胺化反应高区域选择性和对映选择性合成N-取代2-吡啶酮
作者: Zhang X(张霄); Yang ZP(杨泽鹏); Huang L(黄林); You SL(游书力)
通讯作者: 游书力
刊名: Angew. Chem.-Int. Edit.
发表日期: 2015
DOI: 10.1002/anie.201409976
卷: 54, 期:6, 页:1873-1876
收录类别: SCI
文章类型: 论文
英文摘要: The first iridium-catalyzed intermolecular asymmetric allylic amination reaction with 2-hydroxypyridines has been developed, thus providing a highly efficient synthesis of enantioenriched N-substituted 2-pyridone derivatives from readily available starting materials. This protocol features a good tolerance of functional groups in both the allylic carbonates and 2-hydroxypyridines, thereby delivering multifunctionalized heterocyclic products with up to 98% yield and 99%ee.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000349209200035
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39564
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所, 金属有机化学国家重点实验室

Recommended Citation:
Zhang X,Yang ZP,Huang L,et al. Highly Regio- and Enantioselective Synthesis of N-Substituted 2-Pyridones: Iridium-Catalyzed Intermolecular Asymmetric Allylic Amination[J]. Angew. Chem.-Int. Edit.,2015,54(6):1873-1876.
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