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学科主题: 生命有机化学
题名: Total Synthesis of Epoxyeujindole A
其他题名: Total Synthesis of Epoxyeujindole A
作者: Lu ZH(陆钊洪); Li HL(李海龙); Bian M(卞明); Li A(李昂)
通讯作者: 李昂
刊名: J. Am. Chem. Soc.
发表日期: 2015
DOI: 10.1021/jacs.5b09198
卷: 137, 期:43, 页:13764-13767
收录类别: SCI
文章类型: 论文
英文摘要: The total synthesis of epoxyeujindole A, a structurally unusual indole diterpenoid isolated from Eupenicillium javanicum, has been accomplished for the first time. The synthesis features a late-stage cationic cyclization strategy, which took advantage of an electron-rich olefinic substrate. The CDE ring system was assembled via an enantioselective conjugate addition/alkylation, a Luche cyclization, and a Nozaki-Hiyama-Kishi reaction. The heavily substituted A ring was constructed through a Suzuki-Miyaura coupling and a cationic cyclization, and the bridged fused B ring was formed through a Prins reaction.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000364355900011
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39536
Appears in Collections:生命有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所, 生命有机化学国家重点实验室

Recommended Citation:
Lu ZH,Li HL,Bian M,et al. Total Synthesis of Epoxyeujindole A[J]. J. Am. Chem. Soc.,2015,137(43):13764-13767.
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