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学科主题: 生命有机化学
题名: CuI/Oxalic Diamide Catalyzed Coupling Reaction of (Hetero)Aryl Chlorides and Amines
其他题名: 碘化亚铜/草酸二酰胺配体催化的芳基(杂芳基)氯代物与胺的偶联
作者: Zhou W(周伟)1; Fan MY(樊梦阳)1; Yin JL(殷俊力)1; Jiang YW(蒋咏文)1; Ma DW(马大为)1
通讯作者: 马大为
刊名: J. Am. Chem. Soc.
发表日期: 2015
DOI: 10.1021/jacs.5b08411
卷: 137, 期:37, 页:11942-11945
收录类别: SCI
文章类型: 论文
英文摘要: A class of oxalic diamides are found to be effective ligands for promoting CuI-catalyzed aryl amination with less reactive (hetero)aryl chlorides. The reaction proceeds at 120 degrees C with K3PO4 as the base in DMSO to afford a wide range of (hetero)aryl amines in good to excellent yields. The bis(N-aryl) substituted oxalamides are superior ligands to N-aryl-N'-alkyl substituted or bis(N-alkyl) substituted oxalamides. Both the electronic nature and the steric property of the aromatic rings in ligands are important for their efficiency.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000361930000023
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39528
Appears in Collections:生命有机化学国家重点实验室_期刊论文

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作者单位: 1.中科院上海有机化学研究所, 生命有机化学国家重点实验室
2.上海科技大学

Recommended Citation:
Zhou W,Fan MY,Yin JL,et al. CuI/Oxalic Diamide Catalyzed Coupling Reaction of (Hetero)Aryl Chlorides and Amines[J]. J. Am. Chem. Soc.,2015,137(37):11942-11945.
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