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Synthesis of Tricyclo[4,3,1,0(1,5)]decane Core of Plumisclerin A Using Pauson-Khand Annulation and SmI2-Mediated Radical Cyclization
Alternative TitleSynthesis of Tricyclo[4,3,1,0(1,5)]decane Core of Plumisclerin A Using Pauson-Khand Annulation and SmI2-Mediated Radical Cyclization
Chen JP(陈己鹏); He W(何伟); Yang ZY(杨震宇); Yao ZJ(姚祝军)
2015
Source PublicationOrg. Lett.
Volume17Issue:14Pages:3379-3381
AbstractAn efficient synthesis of the tricyclo [4,3,1,0(1,5)]-decane core (B/C/D rings) of plumisclerin A, a unique cytotoxic marine diterpenoid, is described. A Pauson-Khand reaction and a SmI2-mediated radical 1,4-conjugate addition successfully served as key reactions for construction of the fully functionalized 5,6-fused rings and the highly strained cyclobutanol moiety with correct relative stereo chemistries, respectively.
Subtype论文
Subject Area生命有机化学
DOI10.1021/acs.orglett.5b01563
URL查看原文
Indexed BySCI
Language英语
WOS IDWOS:000358395500001
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Document Type期刊论文
Identifierhttp://ir.sioc.ac.cn/handle/331003/39513
Collection生命有机化学国家重点实验室
Corresponding AuthorYao ZJ(姚祝军)
Affiliation中科院上海有机化学研究所, 生命有机化学国家重点实验室
Recommended Citation
GB/T 7714
Chen JP,He W,Yang ZY,et al. Synthesis of Tricyclo[4,3,1,0(1,5)]decane Core of Plumisclerin A Using Pauson-Khand Annulation and SmI2-Mediated Radical Cyclization[J]. Org. Lett.,2015,17(14):3379-3381.
APA 陈己鹏,何伟,杨震宇,&姚祝军.(2015).Synthesis of Tricyclo[4,3,1,0(1,5)]decane Core of Plumisclerin A Using Pauson-Khand Annulation and SmI2-Mediated Radical Cyclization.Org. Lett.,17(14),3379-3381.
MLA 陈己鹏,et al."Synthesis of Tricyclo[4,3,1,0(1,5)]decane Core of Plumisclerin A Using Pauson-Khand Annulation and SmI2-Mediated Radical Cyclization".Org. Lett. 17.14(2015):3379-3381.
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