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学科主题: 生命有机化学
题名: Synthesis of the tetracyclic core of chlorospermines
其他题名: Synthesis of the tetracyclic core of chlorospermines
作者: Wan M(万明)1; Yao M(姚明)1; Gong JY(宫君宇)1; Yang P(杨鹏)1; Liu H(刘华)1; Li A(李昂)1
通讯作者: 刘华 ; 李昂
刊名: Chin. Chem. Lett.
发表日期: 2015
DOI: 10.1016/j.cclet.2015.01.037
卷: 26, 期:3, 页:272-276
收录类别: SCI
文章类型: 论文
英文摘要: Chlorospermines A and B are biologically interesting acridone natural products and recently isolated from Glycosmis chlorosperrna. We report here a convergent approach to construct the tetracyclic core of the natural products. The two fragments are assembled together through Sonogashira coupling, and a cis-triene intermediate was prepared by using hydrosilylation/desilylation. A 6 pi-electrocyclization/aromatization sequence served as the key step of the synthesis, which formed the tetrasubstituted arene motif in one pot. (C) 2015 Hua Liu and Ang Li. Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences. All rights reserved.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000353089000002
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39498
Appears in Collections:生命有机化学国家重点实验室_期刊论文

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作者单位: 1.江西中医药大学
2.中科院上海有机化学研究所, 生命有机化学国家重点实验室

Recommended Citation:
Wan M,Yao M,Gong JY,et al. Synthesis of the tetracyclic core of chlorospermines[J]. Chin. Chem. Lett.,2015,26(3):272-276.
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