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A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates
Alternative Title手性膦催化的碳、氮-环状亚胺和δ-取代联烯酸酯的[3+2]不对称反应环加成反应
Wang D(王德); Lei Y(雷煜); Wei Y(魏音); Shi M(施敏)
2014
Source PublicationChem.-Eur. J.
Volume20Issue:47Pages:15325-15329
AbstractCatalytic asymmetric [3+2] cycloadditions of C,N-cyclic azomethine imines with delta-substituted allenoates have been developed in the presence of (S)-Me-f-Ketal-Phos, affording functionalized tetrahydroquinoline frameworks in good yields with high diastereo- and good enantioselectivities under mild condition. The substrate scope has been also examined. This is the first time that delta-substituted allenoates have been applied as delta,gamma-C-C bond participated C-2 synthon in asymmetric synthesis.
Subject Area金属有机化学
DOI10.1002/chem.201405191
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Indexed BySCI
Language英语
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Cited Times:51[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sioc.ac.cn/handle/331003/39131
Collection金属有机化学国家重点实验室
Corresponding AuthorShi M(施敏)
Affiliation中科院上海有机化学研究所
Recommended Citation
GB/T 7714
Wang D,Lei Y,Wei Y,et al. A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates[J]. Chem.-Eur. J.,2014,20(47):15325-15329.
APA 王德,雷煜,魏音,&施敏.(2014).A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates.Chem.-Eur. J.,20(47),15325-15329.
MLA 王德,et al."A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates".Chem.-Eur. J. 20.47(2014):15325-15329.
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