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学科主题: 金属有机化学
题名: A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates
其他题名: 手性膦催化的碳、氮-环状亚胺和δ-取代联烯酸酯的[3+2]不对称反应环加成反应
作者: Wang D(王德); Lei Y(雷煜); Wei Y(魏音); Shi M(施敏)
通讯作者: 施敏
刊名: Chem.-Eur. J.
发表日期: 2014
DOI: 10.1002/chem.201405191
卷: 20, 期:47, 页:15325-15329
收录类别: SCI
英文摘要: Catalytic asymmetric [3+2] cycloadditions of C,N-cyclic azomethine imines with delta-substituted allenoates have been developed in the presence of (S)-Me-f-Ketal-Phos, affording functionalized tetrahydroquinoline frameworks in good yields with high diastereo- and good enantioselectivities under mild condition. The substrate scope has been also examined. This is the first time that delta-substituted allenoates have been applied as delta,gamma-C-C bond participated C-2 synthon in asymmetric synthesis.
语种: 英语
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39131
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所

Recommended Citation:
Wang D,Lei Y,Wei Y,et al. A Phosphine-Catalyzed Novel Asymmetric [3+2] Cycloaddition of C,N-Cyclic Azomethine Imines with delta-Substituted Allenoates[J]. Chem.-Eur. J.,2014,20(47):15325-15329.
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