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Insertion of Nitriles into Zirconocene 1-aza-1,3-diene Complexes: Chemoselective Synthesis of N-H and N-Substituted Pyrroles
Alternative TitleInsertion of Nitriles into Zirconocene 1-aza-1,3-diene Complexes: Chemoselective Synthesis of N-H and N-Substituted Pyrroles
YU SHASHA; XIONG MEIJUN; XIE XIN; Liu YH(刘元红)
2014
Source PublicationAngew. Chem.-Int. Edit.
Volume53Issue:43Pages:11596-11599
AbstractThe direct insertion of nitriles into zirconocene-1-aza-1,3-diene complexes provides an efficient, chemoselective, and controllable synthesis of N-H and N-substituted pyrroles upon acidic aqueous work-up. The outcome of the reaction (that is, the formation of N-H or N-substituted pyrroles) results from the different cyclization patterns, which depend on the relative stability and reactivity of the enamine-imine tautomers formed by hydrolysis of the diazazirconacycles.
Subject Area金属有机化学
DOI10.1002/anie.201407221
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Indexed BySCI
Language英语
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Cited Times:19[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sioc.ac.cn/handle/331003/39118
Collection金属有机化学国家重点实验室
Affiliation中科院上海有机化学研究所
Recommended Citation
GB/T 7714
YU SHASHA,XIONG MEIJUN,XIE XIN,et al. Insertion of Nitriles into Zirconocene 1-aza-1,3-diene Complexes: Chemoselective Synthesis of N-H and N-Substituted Pyrroles[J]. Angew. Chem.-Int. Edit.,2014,53(43):11596-11599.
APA YU SHASHA,XIONG MEIJUN,XIE XIN,&刘元红.(2014).Insertion of Nitriles into Zirconocene 1-aza-1,3-diene Complexes: Chemoselective Synthesis of N-H and N-Substituted Pyrroles.Angew. Chem.-Int. Edit.,53(43),11596-11599.
MLA YU SHASHA,et al."Insertion of Nitriles into Zirconocene 1-aza-1,3-diene Complexes: Chemoselective Synthesis of N-H and N-Substituted Pyrroles".Angew. Chem.-Int. Edit. 53.43(2014):11596-11599.
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