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学科主题: 金属有机化学
题名: Kinetic Resolution of 2-Substituted 2,3-Dihydro-4-pyridones by Palladium-Catalyzed Asymmetric Allylic Alkylation: Catalytic Asymmetric Total Synthesis of Indolizidine (-)-209I
其他题名: 钯催化烯丙基取代反应对2-取代-2,3-二氢哌啶酮的动力学拆分: Indizidine (-)-209I 的催化不对称全合成
作者: Lei BL(雷柏林); Zhang QS(张卿菘); Yu WH(余伟华); Ding QP(丁秋平); Ding CH(丁昌华); Hou XL(侯雪龙)
通讯作者: 丁昌华 ; 侯雪龙
刊名: Org. Lett.
发表日期: 2014
DOI: 10.1021/ol500498m
卷: 16, 期:7, 页:1944-1947
收录类别: SCI
英文摘要: The kinetic resolution of 2-substituted-2,3-dihydro-4-pyridones was realized via a Pd-catalyzed allylic substitution reaction using a commercially available (S)-P-Phos as a ligand, affording optically active dihydropyridones and C-allylated dihydropyridones in high yields and good enantioselectivities with the S-factor up to 43. With this protocol, a catalytic asymmetric total synthesis of indolizidine (-)-209I was realized for the first time.
语种: 英语
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/39050
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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作者单位: 中科院上海有机化学研究所

Recommended Citation:
Lei BL,Zhang QS,Yu WH,et al. Kinetic Resolution of 2-Substituted 2,3-Dihydro-4-pyridones by Palladium-Catalyzed Asymmetric Allylic Alkylation: Catalytic Asymmetric Total Synthesis of Indolizidine (-)-209I[J]. Org. Lett.,2014,16(7):1944-1947.
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