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Bioinspired Total Synthesis of Sespenine
Alternative TitleBioinspired Total Synthesis of Sespenine
Sun Y(孙域)1; Chen PX(陈鹏西)1; Zhang DL(张德良)1; BAUNACH MARTIN1; HERTWECK CHRISTIAN1; Li A(李昂)1
Source PublicationAngew. Chem.-Int. Edit.
AbstractThe first total synthesis of sespenine, a rare indole sesquiterpenoid from a mangrove endophyte, has been accomplished. A bioinspired aza-Prins/Friedel-Crafts/retro Friedel-Crafts cascade reaction assembles the bridged tetrahydroquinoline core. Further investigations on the aza-Prins cyclization imply that the C3 configuration of the hydroxyindolenine intermediate is crucial to the biosynthesis of sespenine and its congener xiamycin A.
Subject Area生命有机化学
Indexed BySCI
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Cited Times:46[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Corresponding AuthorLi A(李昂)
Recommended Citation
GB/T 7714
Sun Y,Chen PX,Zhang DL,et al. Bioinspired Total Synthesis of Sespenine[J]. Angew. Chem.-Int. Edit.,2014,53(34):9012-9016.
APA 孙域,陈鹏西,张德良,BAUNACH MARTIN,HERTWECK CHRISTIAN,&李昂.(2014).Bioinspired Total Synthesis of Sespenine.Angew. Chem.-Int. Edit.,53(34),9012-9016.
MLA 孙域,et al."Bioinspired Total Synthesis of Sespenine".Angew. Chem.-Int. Edit. 53.34(2014):9012-9016.
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