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Total Synthesis of Taiwaniadducts B, C, and D
Alternative TitleTotal Synthesis of Taiwaniadducts B, C, and D
Deng J(邓军); Zhou SP(周述鹏); Zhang WH(张纹豪); Li J(李健); Li RF(李若凡); Li A(李昂)
Source PublicationJ. Am. Chem. Soc.
AbstractThe first total syntheses of taiwaniadducts B, C, and D have been accomplished. Two diterpenoid segments were prepared with high enantiopurity, both through Ir-catalyzed asymmetric polyene cyclization. A sterically demanding intermolecular Diels-Alder reaction promoted by Er(fod)(3) assembled the scaffold of taiwaniadducts B and C. A carbonyl-ene cyclization forged the cage motif of taiwaniadduct D at a late stage, providing over 200 mg of this compound.
Subject Area生命有机化学
Indexed BySCI
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Document Type期刊论文
Corresponding AuthorLi A(李昂)
Recommended Citation
GB/T 7714
Deng J,Zhou SP,Zhang WH,et al. Total Synthesis of Taiwaniadducts B, C, and D[J]. J. Am. Chem. Soc.,2014,136(23):8185-8188.
APA 邓军,周述鹏,张纹豪,李健,李若凡,&李昂.(2014).Total Synthesis of Taiwaniadducts B, C, and D.J. Am. Chem. Soc.,136(23),8185-8188.
MLA 邓军,et al."Total Synthesis of Taiwaniadducts B, C, and D".J. Am. Chem. Soc. 136.23(2014):8185-8188.
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