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学科主题: 天然产物有机化学
题名: Total Synthesis of (-)-Fusarisetin A and Reassignment of the Absolute Configuration of Its Natural Counterpart
其他题名: (?)-Fusarisetin A的全合成及其绝对构型的更正
作者: Deng J(邓军) ; Zhu B(朱波) ; Lu ZY(鲁照永) ; Yu HX(于海昕) ; Li A(李昂)
通讯作者: 李昂
刊名: J. Am. Chem. Soc.
发表日期: 2012
卷: 134, 期:2, 页:920-923
收录类别: SCI
部门归属: 中科院上海有机化学研究所
英文摘要: The first total synthesis of (-)-fusarisetin A, the enantiomer of naturally occurring acinar morphogenesis inhibitor (+)-fusarisetin A, was accomplished in 13 steps, leading to the reassignment of the absolute configuration of the natural product. The synthesis featured a Lewis acid-promoted intramolecular Diets-Alder reaction, a Pd-catalyzed O -> C allylic rearrangement, a chemoselective Wacker oxidation, and a Dieckmann condensation/hemiketalization cascade.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000301084300046
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/28613
Appears in Collections:中科院天然产物有机化学重点实验室_期刊论文

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Recommended Citation:
Deng J,Zhu B,Lu ZY,et al. Total Synthesis of (-)-Fusarisetin A and Reassignment of the Absolute Configuration of Its Natural Counterpart[J]. J. Am. Chem. Soc.,2012,134(2):920-923.
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