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Use of Side-Chain Incompatibility for Tailoring Long-Range p/n Heterojunctions: Photoconductive Nanofibers Formed by Self-Assembly of an Amphiphilic Donor-Acceptor Dyad Consisting of Oligothiophene and Perylenediimide
其他题名应用侧链的不相容性调控长距离的p/n异质结: 光电导性纳米纤维形成于两亲含寡聚噻吩和苝酰亚胺的给-受体二元体系化合物的自组装
Li WS(李维实); SAEKI AKINORI; YAMAMOTO YOHEI; FUKUSHIMA TAKANORI; SEKI SHU; ISHII NORIYUKI; KATO KENICHI; TAKATA MASAKI; AIDA TAKUZO
2010
发表期刊Chem.-Asian J.
ISSN1861-4728
卷号5期号:7页码:1566-1572
摘要To tailor organic p/n heterojunctions with molecular-level precision, a rational design strategy using side-chain incompatibility of a covalently connected donor acceptor (D-A) dyad has been successfully carried out. An oligothiophene-perylenediimide dyad, when modified with triethylene glycol side chains at one terminus and dodecyl side chains at the other (2(Amphi)), self-assembles into nanofibers with a long-range D/A heterojunction. In contrast, when the dyad is modified with dodecyl side chains at both termini (214), ill-defined microfibers result. In steady-state measurements using microgap electrodes, a cast film of the nanofiber of 2(Amphi) displays far better photoconducting properties than that of the microfiber of 2(Lipo).. Flash-photolysis time-resolved microwave conductivity measurements, in conjunction with transient absorption spectroscopy, clearly indicate that the nanofiber of 2(Amphi) intrinsically allows for better carrier generation and transport properties than the microfibrous assembly of 2(Lipo).
学科领域高分子化学
部门归属中国科学院上海有机化学研究所; 日本大阪大学; 日本学术振兴机构; 日本理化研究所; 日本东京大学
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收录类别SCI
语种英语
WOS记录号WOS:000280869300008
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被引频次:44[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.sioc.ac.cn/handle/331003/28377
专题高分子材料研究室
通讯作者Li WS(李维实); FUKUSHIMA TAKANORI; AIDA TAKUZO
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Li WS,SAEKI AKINORI,YAMAMOTO YOHEI,et al. Use of Side-Chain Incompatibility for Tailoring Long-Range p/n Heterojunctions: Photoconductive Nanofibers Formed by Self-Assembly of an Amphiphilic Donor-Acceptor Dyad Consisting of Oligothiophene and Perylenediimide[J]. Chem.-Asian J.,2010,5(7):1566-1572.
APA 李维实.,SAEKI AKINORI.,YAMAMOTO YOHEI.,FUKUSHIMA TAKANORI.,SEKI SHU.,...&AIDA TAKUZO.(2010).Use of Side-Chain Incompatibility for Tailoring Long-Range p/n Heterojunctions: Photoconductive Nanofibers Formed by Self-Assembly of an Amphiphilic Donor-Acceptor Dyad Consisting of Oligothiophene and Perylenediimide.Chem.-Asian J.,5(7),1566-1572.
MLA 李维实,et al."Use of Side-Chain Incompatibility for Tailoring Long-Range p/n Heterojunctions: Photoconductive Nanofibers Formed by Self-Assembly of an Amphiphilic Donor-Acceptor Dyad Consisting of Oligothiophene and Perylenediimide".Chem.-Asian J. 5.7(2010):1566-1572.
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