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学科主题: 金属有机化学
题名: Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds
其他题名: Rh(I)催化的亚乙烯基环丙烷和CO的[3+2+1]P-K类型环化反应: 一个高区域和高立体选择性合成氮或氧杂双环化合物的新方法
作者: Lu BL(卢贝丽) ; Wei Y(魏音) ; Shi M(施敏)
通讯作者: 施敏
刊名: Organometallics
发表日期: 2012
卷: 31, 期:12, 页:4601-4609
收录类别: SCI
部门归属: 中科院上海有机化学研究所
英文摘要: In this paper, a novel Rh(I)-catalyzed Pauson-Khand-type [3 + 2 + 1] cycloaddition reaction of ene-vinylidenecyclopropanes (Ene-VDCPs) and carbon monoxide (CO) has been developed to furnish a series of aza- and oxa-bicyclic compounds in moderate to good yields in a highly regio- and diastereoselective manner, which provides an alternative and efficient synthetic approach for the access of bicyclic cyclohexanone frameworks. The substrate scope and limitations and a plausible mechanism are discussed.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000305588000028
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/27961
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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Recommended Citation:
Lu BL,Wei Y,Shi M. Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds[J]. Organometallics,2012,31(12):4601-4609.
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