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Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds
其他题名Rh(I)催化的亚乙烯基环丙烷和CO的[3+2+1]P-K类型环化反应: 一个高区域和高立体选择性合成氮或氧杂双环化合物的新方法
Lu BL(卢贝丽); Wei Y(魏音); Shi M(施敏)
2012
发表期刊Organometallics
ISSN0276-7333
卷号31期号:12页码:4601-4609
摘要In this paper, a novel Rh(I)-catalyzed Pauson-Khand-type [3 + 2 + 1] cycloaddition reaction of ene-vinylidenecyclopropanes (Ene-VDCPs) and carbon monoxide (CO) has been developed to furnish a series of aza- and oxa-bicyclic compounds in moderate to good yields in a highly regio- and diastereoselective manner, which provides an alternative and efficient synthetic approach for the access of bicyclic cyclohexanone frameworks. The substrate scope and limitations and a plausible mechanism are discussed.
学科领域金属有机化学
部门归属中科院上海有机化学研究所
URL查看原文
收录类别SCI
语种英语
WOS记录号WOS:000305588000028
引用统计
被引频次:19[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.sioc.ac.cn/handle/331003/27961
专题金属有机化学国家重点实验室
通讯作者Shi M(施敏)
推荐引用方式
GB/T 7714
Lu BL,Wei Y,Shi M. Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds[J]. Organometallics,2012,31(12):4601-4609.
APA 卢贝丽,魏音,&施敏.(2012).Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds.Organometallics,31(12),4601-4609.
MLA 卢贝丽,et al."Rhodium(I)-Catalyzed Pauson-Khand-type [3+2+1] Cycloaddition Reaction of Ene-Vinylidenecyclopropanes and CO: A Highly Regio- and Stereoselective Synthetic Approach for the Preparation of Aza- and Oxa-Bicyclic Compounds".Organometallics 31.12(2012):4601-4609.
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