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学科主题: 金属有机化学
题名: Bronsted Base-Modulated Regioselective Pd-Catalyzed Intramolecular Aerobic Oxidative Amination of Alkenes: Formation of Seven-Membered Amides and Evidence for Allylic C-H Activation
其他题名: Bronsted Base-Modulated Regioselective Pd-Catalyzed Intramolecular Aerobic Oxidative Amination of Alkenes: Formation of Seven-Membered Amides and Evidence for Allylic C-H Activation
作者: Wu L(吴亮) ; Qiu SF(邱水发) ; Liu GS(刘国生)
通讯作者: 刘国生
刊名: Org. Lett.
发表日期: 2009
卷: 11, 期:12, 页:2707-2710
收录类别: SCI
部门归属: 上海有机所
英文摘要: A novel palladium-catalyzed intramolecular aerobic oxidative allylic C-H amination of olefins has been developed. Bronsted base can modulate the regioselectivity, favoring the formation of 7-membered rings. Mechanistic studies using deuterium-labeled substrates as probes support a rate-determining allylic C-H activation/irreversible reductive elimination pathway.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000266930900058
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/27871
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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Recommended Citation:
Wu L,Qiu SF,Liu GS. Bronsted Base-Modulated Regioselective Pd-Catalyzed Intramolecular Aerobic Oxidative Amination of Alkenes: Formation of Seven-Membered Amides and Evidence for Allylic C-H Activation[J]. Org. Lett.,2009,11(12):2707-2710.
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