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学科主题: 高分子化学
题名: Polyallene-based graft copolymer via 6-methyl-1,2-heptadien-4-ol and methyl methacrylate
其他题名: 以6-甲基-1,2-庚二烯-4-醇和甲基丙烯酸甲酯为单体合成聚联烯主链的接枝共聚物
作者: Zhang XH(张晓环) ; Shen Z(沈重) ; Li LT(李利涛) ; Lu GL(陆国林) ; Gu LN(顾丽娜) ; Huang XY(黄晓宇)
通讯作者: 黄晓宇
刊名: Polymer
发表日期: 2007
卷: 48, 期:19, 页:5507-5513
收录类别: SCI
部门归属: 上海有机化学研究所
英文摘要: A series of well-defined graf:: copolymers with a polyallene-based backbone and poly(methyl methacrylate) side chains were synthesized by the combination of living coordination polymerization of 6-methyl- 1,2-heptadien-4-ol and atom transfer radical polymerization of methyl methacrylate. We first prepared poly(alcohol) with polyallene repeating units via 6-methyl-1,2-heptadien-4-ol by living coordination polymerization initiated by [(eta(3)-allyl)NiOCOCF3](2), followed by transforming the pendant hydroxyl groups into halogen-containing ATRP initiation groups. Next, grafting-from route was used for the synthesis of the well-defined graft copolymer with excellent solubility: poly(methyl methacrylate) was grafted to the backbone via ATRP of methyl methacrylate. This kind of graft copolymer is the first example of graft copolymer via allene derivative and methacrylic monomer. (C) 2007 Elsevier Ltd. All rights reserved.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000250161000008
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/24375
Appears in Collections:高分子材料研究室_期刊论文

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Recommended Citation:
Zhang XH,Shen Z,Li LT,et al. Polyallene-based graft copolymer via 6-methyl-1,2-heptadien-4-ol and methyl methacrylate[J]. Polymer,2007,48(19):5507-5513.
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