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学科主题: 分析化学
题名: Studies of the Interesting Gas-phase Rearrangement Reactions of 2-Pyrimidinyloxy-N-arylbenzylurea Promoted by Urea-Carbamimidic Acid Tautomerism by ESI-MS/MS and Theoretical Computation
其他题名: ESI-MS/MS结合理论计算研究有趣的 Urea-Carbamimidic Acid Tautomerism引起的 2-Pyrimidinyloxy-N-arylbenzylurea气相重排反应
作者: Xu C(许楚) ; Wang HY(王昊阳) ; Zhao ZX(赵志雄) ; Tang QH(唐庆红) ; Guo YL(郭寅龙) ; Lv L(吕龙)
通讯作者: 郭寅龙 ; 吕龙
刊名: Chin. J. Chem.
发表日期: 2010
卷: 28, 期:9, 页:1765-1772
收录类别: SCI
部门归属: 中国科学院上海有机化学研究所
英文摘要: The gas-phase rearrangement reactions of compound 1, 2-dimethoxypyrimidinyloxybenzylaminobenzenedipropylurea, were studied by ESI-MS/MS. The experimental results showed that introduction of dipropylurea moiety into the molecule initiated various interesting gas-phase chemistries and the mechanisms were proposed on the basis of hydrogen/deuterium (H/D) exchange experiments and theoretical computations. Moreover, product 2, the solution-phase rearrangement product of compound 1, was synthesized and its gas-phase chemistries were also studied to support the propos gas-phase rearrangement reactions of compound 1.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000282998700041
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/20006
Appears in Collections:分析化学研究室_期刊论文

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Recommended Citation:
Xu C,Wang HY,Zhao ZX,et al. Studies of the Interesting Gas-phase Rearrangement Reactions of 2-Pyrimidinyloxy-N-arylbenzylurea Promoted by Urea-Carbamimidic Acid Tautomerism by ESI-MS/MS and Theoretical Computation[J]. Chin. J. Chem.,2010,28(9):1765-1772.
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