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学科主题: 金属有机化学
题名: An Organocatalytic Asymmetric Tandem Reaction for the Construction of Bicyclic Skeletons
其他题名: An Organocatalytic Asymmetric Tandem Reaction for the Construction of Bicyclic Skeletons
作者: Cao CL(曹春利) ; Zhou YY(周友运) ; Zhou J(周剑) ; Sun XL(孙秀丽) ; Tang Y(唐勇) ; Li YX(李玉学) ; Li GY(李光玉) ; Sun J(孙杰)
通讯作者: 唐勇 ; 李玉学
刊名: Chem.-Eur. J.
发表日期: 2009
卷: 15, 期:42, 页:11384-11389
收录类别: SCI
部门归属: 上海有机所
英文摘要: Cyclic ketones react with (E)-2-nitroallylic acetates in the presence of catalytic pyrrolidine-thiourea, which affords bicyclic skeletons with four or five stereocenters in one single reaction with up to 98% ee in moderate to high yields. The cooperative effects of both enamine and the Bronsted acid are found to be crucial for the high reactivity and enantioselectivity of this cascade reaction, which is demonstrated by both theoretical calculation and experimental data.
语种: 英语
相关网址: 查看原文
WOS记录号: WOS:000271560000039
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内容类型: 期刊论文
URI标识: http://ir.sioc.ac.cn/handle/331003/19357
Appears in Collections:金属有机化学国家重点实验室_期刊论文

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Recommended Citation:
Cao CL,Zhou YY,Zhou J,et al. An Organocatalytic Asymmetric Tandem Reaction for the Construction of Bicyclic Skeletons[J]. Chem.-Eur. J.,2009,15(42):11384-11389.
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