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Unexpected dramatic substituent effect for tuning the selectivity in the double ring-closing metathesis reaction of N-containing tetraenes. An efficient synthesis of bicyclic izidine alkaloid skeletons
Alternative Title含氮四烯的双关环复分解反应中的取代基效应 Izidine Alkaloid骨架的有效合成
Ma SM(麻生明); Ni BK(倪步阔)
2002
Source PublicationOrg. Lett.
ISSN1523-7060
Volume4Issue:4Pages:639-641
AbstractA double ring-closing metathesis reaction for the efficient construction of the fused bicyclic izidine alkaloid skeleton was developed. In this reaction, high selectivity was realized by tuning of electronic and steric effects of substituents in the N_containing tetraenes. It was observed that the reactivity of electron-rich carbon-carbon double bonds in higher than that of electron-deficient ones. A brief mechanistic study is also discussed.
Subject Area有机化学
Department中国科学院上海有机化学研究所金属有机化学开放实验室
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Indexed BySCI
Language英语
WOS IDWOS:000173885800043
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Document Type期刊论文
Identifierhttp://ir.sioc.ac.cn/handle/331003/11878
Collection金属有机化学国家重点实验室
Corresponding AuthorMa SM(麻生明)
Recommended Citation
GB/T 7714
Ma SM,Ni BK. Unexpected dramatic substituent effect for tuning the selectivity in the double ring-closing metathesis reaction of N-containing tetraenes. An efficient synthesis of bicyclic izidine alkaloid skeletons[J]. Org. Lett.,2002,4(4):639-641.
APA 麻生明,&倪步阔.(2002).Unexpected dramatic substituent effect for tuning the selectivity in the double ring-closing metathesis reaction of N-containing tetraenes. An efficient synthesis of bicyclic izidine alkaloid skeletons.Org. Lett.,4(4),639-641.
MLA 麻生明,et al."Unexpected dramatic substituent effect for tuning the selectivity in the double ring-closing metathesis reaction of N-containing tetraenes. An efficient synthesis of bicyclic izidine alkaloid skeletons".Org. Lett. 4.4(2002):639-641.
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